If you've verified the preshared key and it's still giving that error,
1.) Confirm that you have the controller listed as a RADIUS client on the second NPS server.
2.) Make sure the RADIUS policy is enabled for the EAP type you're using (e.g. PEAP).
3.) If you're using a server side certificate, make sure the correct one is selected for that policy.
Hope this helps!
- Jay